Meat Puppets. I had heard of them on the Nirvana Unplugged album, but didn't listen to them until about 5 years ago.
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The Flaming Lips.
I knew about them in my teens, but I never really got in to them. Then The Soft Bulletin came out in 1999 and I immediately became a fan.
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Also, the Faces (courtesy of Black Crowes covering them). Never heard of them before 2005, and thought Rod Stewart only put out crappy 80's stuff. Loosest rock and roll I've heard. Good stuff.